Plasma-catalytic oxidation of adsorbed toluene on Ag–Mn/γ-Al2O3: Comparison of gas flow-through and gas circulation treatment.
发布时间:2024-08-09
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- 所属单位:
- 环境与市政工程学院
- 发表刊物:
- Chemical Engineering Journal
- 关键字:
- 中文关键字:低温等离子体;气体直流;气体循环;,英文关键字:Non-thermal plasma;Gas flow-through;Gas circulatio
- 摘要:
- Oxidation of adsorbed toluene was investigated in a dielectric barrier discharge reactor at atmospheric pressure coupled with Ag–Mn/c-Al2O3 catalysts. Gas flow-through and gas circulation systems were compared in the same reactor with the same operating conditions. After 90 min of plasma treatment, the mineralization of adsorbed toluene reached 68% in the O2 flow-through system with some emission of desorbed toluene. For the O2 circulation system, the mineralization of adsorbed toluene increased to 78% without any emission of desorbed toluene. Furthermore, compared to the gas flow-through system, the CO2 selectivity in the gas circulation system was improved in both air and oxygen plasma. Moreover, the circulation system was more efficient than the gas flow-through system for O3 decomposition, resulting in better mineralization of adsorbed toluene and CO2 selectivity.
- 备注:
- 通讯作者:党小庆
- 合写作者:
- 黄家玉,腾晶晶
- 第一作者:
- 黄学敏,党小庆,秦彩虹
- 论文类型:
- 期刊论文
- 卷号:
- 卷:299
- 期号:
- 期:
- 页面范围:
- 页:85–92
- 是否译文:
- 否
- 发表时间:
- 2016-12-01